A Comprehensive Review on the Recycling of Carbon Fibre–Reinforced Polymer Composite: Recovery Techniques, Material Performance, and Sustainability
Main Article Content
Article Details
References
[1]Kaufmann, J. (2015). New materials for sports equipment made of anisotropic fiber-reinforced plastics with stiffness related coupling effect. Procedia Engineering, 112, 140–145. https://doi.org/10.1016/j.proeng.2015.07.189
[2]Mallick, P. K. (2007). Fiber-reinforced composites: Materials, manufacturing, and design (3rd ed.). CRC Press. https://doi.org/10.1201/9781420005981
[3]Marsh, G. (2010). Airbus A350 XWB update. Reinforced Plastics, 54(6), 20–24. https://doi.org/10.1016/S0034-3617(10)70212-5
[4]Jacob, A. (2014). Carbon fibre and cars – 2013 in review. Reinforced Plastics, 58(1), 18–19. https://doi.org/10.1016/S0034-3617(14)70036-0
[5]Kaufmann, J., Rabe, H., Siebert, N., Wolf, P., Cebulla, H., & Odenwald, S. (2016). Smart carbon fiber bicycle seat post with light and sensor integration. Procedia Engineering, 147, 562–567. https://doi.org/10.1016/j.proeng.2016.06.239
[6]Brøndsted, P., Lilholt, H., & Lystrup, A. (2005). Composite materials for wind power turbine blades. Annual Review of Materials Research, 35, 505–538. https://doi.org/10.1146/annurev.matsci.35.100303.110641
[7]Holmes, M. (2014). Global carbon fibre market remains on upward trend. Reinforced Plastics, 58(6), 38–45. https://doi.org/10.1016/S0034-3617(14)70251-6
[8]Red, C. (2008). Wind turbine blades: Big and getting bigger. Composites Technology, 14(3), 42–47.
[9]Pickering, S. J. (2006). Recycling technologies for thermoset composite materials—current status. Composites Part A: Applied Science and Manufacturing, 37(8), 1206–1215. https://doi.org/10.1016/j.compositesa.2005.05.030
[10]Oliveux, G., Dandy, L. O., & Leeke, G. A. (2015). Current status of recycling of fibre reinforced polymers: Review of technologies, reuse and resulting properties. Progress in Materials Science, 72, 61–99. https://doi.org/10.1016/j.pmatsci.2015.01.004
[11]Liu, P., & Barlow, C. Y. (2017). Wind turbine blade waste in 2050. Waste Management, 62, 229–240. https://doi.org/10.1016/j.wasman.2017.02.007
[12]Reinhardt, M., Kaufmann, J., Kausch, M., & Kroll, L. (2013). PLA-viscose-composites with continuous fibre reinforcement for structural applications. Procedia Materials Science, 2, 137–143. https://doi.org/10.1016/j.mspro.2013.02.016
[13]Schmidt, J., Klingenhöfer, M., Kaufmann, J., Cebulla, H., & Kroll, L. (2021). Characterization of the interlaminar fracture toughness of unidirectional thermoplastic composites. Technologies for Lightweight Structures, 5(1), 69–77. https://doi.org/10.21935/tls.v5i1.157
[14]Yang, Y., Boom, R., Irion, B., van Heerden, D.-J., Kuiper, P., & de Wit, H. (2012). Recycling of composite materials. Chemical Engineering and Processing: Process Intensification, 51, 53–68. https://doi.org/10.1016/j.cep.2011.09.007
[15]Naqvi, S. R., Prabhakara, H. M., Bramer, E. A., Dierkes, W., Akkerman, R., & Brem, G. (2018). A critical review on recycling of end-of-life carbon fibre/glass fibre reinforced composites waste using pyrolysis towards a circular economy. Resources, Conservation and Recycling, 136, 118–129. https://doi.org/10.1016/j.resconrec.2018.04.013
[16]Ribeiro, I., Kaufmann, J., Schmidt, A., Peças, P., Henriques, E., & Götze, U. (2016). Fostering selection of sustainable manufacturing technologies: A case study involving product design, supply chain and life cycle performance. Journal of Cleaner Production, 112, 3306–3319. https://doi.org/10.1016/j.jclepro.2015.10.043
[17]Song, Y. S., Youn, J. R., & Gutowski, T. G. (2009). Life cycle energy analysis of fiber-reinforced composites. Composites Part A: Applied Science and Manufacturing, 40(8), 1257–1265. https://doi.org/10.1016/j.compositesa.2009.05.020
[18]Karuppannan Gopalraj, S., & Kärki, T. (2020). A review on the recycling of waste carbon fibre/glass fibre-reinforced composites: Fibre recovery, properties and life-cycle analysis. SN Applied Sciences, 2, Article 433. https://doi.org/10.1007/s42452-020-2195-4
[19]European Parliament & Council of the European Union. (2008). Directive 2008/98/EC of the European Parliament and of the Council of 19 November 2008 on waste and repealing certain Directives. Official Journal of the European Union, L 312, 3–30.
[20]U.S. Environmental Protection Agency. (2019). Resource Conservation and Recovery Act (RCRA) overview. https://www.epa.gov/rcra/resource-conservation-and-recovery-act-rcra-overview.
[21]Zhang, J., Chevali, V. S., Wang, H., & Wang, C.-H. (2020). Current status of carbon fibre and carbon fibre composites recycling. Composites Part B: Engineering, 193, Article 108053. https://doi.org/10.1016/j.compositesb.2020.108053
[22]Holmes, M. (2013). Carbon fibre reinforced plastics market continues growth path. Reinforced Plastics, 57(6), 24–29. https://doi.org/10.1016/S0034-3617(13)70186-3
[23]Meng, F., Olivetti, E. A., Zhao, Y., Chang, J. C., Pickering, S. J., & McKechnie, J. (2018). Comparing life cycle energy and global warming potential of carbon fiber composite recycling technologies and waste management options. ACS Sustainable Chemistry & Engineering, 6(8), 9854–9865. https://doi.org/10.1021/acssuschemeng.8b01026
[24]Kaufmann, J., Kroll, L., & Odenwald, S. (2010). Application-specific design of sports equipment from anisotropic fiber-reinforced plastics with stiffness related coupling effect. Procedia Engineering, 2(2), 2569–2574. https://doi.org/10.1016/j.proeng.2010.04.033
[25]Morgan, P. (2005). Carbon fibers and their composites. CRC Press. https://doi.org/10.1201/9781420028744
[26]Fitzer, E. (1989). Pan-based carbon fibers—Present state and trend of the technology from the viewpoint of possibilities and limits to influence and to control the fiber properties by the process parameters. Carbon, 27(5), 621–645. https://doi.org/10.1016/0008-6223(89)90197-8
[27]Toray Industries, Inc. (2023). Torayca carbon fiber: Technical data sheet.
[28]Guigon, M., Oberlin, A., & Desarmot, G. (1984). Microtexture and structure of some high tensile strength, PAN-base carbon fibers. Fibre Science and Technology, 20(1), 55–72. https://doi.org/10.1016/0015-0568(84)90057-5
[29]Ellis, B. (Ed.). (1993). Chemistry and technology of epoxy resins. Blackie Academic & Professional.
[30]May, C. A. (Ed.). (1988). Epoxy resins: Chemistry and technology (2nd ed., rev. and expanded). Marcel Dekker.
[31]Pascault, J.-P., Sautereau, H., Verdu, J., & Williams, R. J. J. (2002). Thermosetting polymers. Marcel Dekker.
[32]Biron, M. (2013). Thermoplastics and thermoplastic composites (2nd ed.). Elsevier.
[33]Drzal, L. T. (1986). The interphase in epoxy composites. In K. Dušek (Ed.), Epoxy resins and composites II (pp. 1–32). Springer. https://doi.org/10.1007/BFb0017913
[34]Jones, C. (1991). The chemistry of carbon fibre surfaces and its effect on interfacial phenomena in fibre/epoxy composites. Composites Science and Technology, 42(1–3), 275–298. https://doi.org/10.1016/0266-3538(91)90021-G
[35]Rybicka, J., Tiwari, A., & Leeke, G. A. (2016). Technology readiness level assessment of composites recycling technologies. Journal of Cleaner Production, 112(Part 1), 1001–1012. https://doi.org/10.1016/j.jclepro.2015.08.104
[36]Krauklis, A. E., Karl, C. W., Gagani, A. I., & Jørgensen, J. K. (2021). Composite material recycling technology—State-of-the-art and sustainable development for the 2020s. Journal of Composites Science, 5(1), Article 28. https://doi.org/10.3390/jcs5010028
[37]Howarth, J., Mareddy, S. S. R., & Mativenga, P. T. (2014). Energy intensity and environmental analysis of mechanical recycling of carbon fibre composite. Journal of Cleaner Production, 81, 46–50. https://doi.org/10.1016/j.jclepro.2014.06.023
[38]Shuaib, N. A., & Mativenga, P. T. (2016). Energy demand in mechanical recycling of glass fibre reinforced thermoset plastic composites. Journal of Cleaner Production, 120, 198–206. https://doi.org/10.1016/j.jclepro.2016.01.070
[39]Pickering, S. J., Kelly, R. M., Kennerley, J. R., Rudd, C. D., & Fenwick, N. J. (2000). A fluidised-bed process for the recovery of glass fibres from scrap thermoset composites. Composites Science and Technology, 60(4), 509–523. https://doi.org/10.1016/S0266-3538(99)00154-2
[40]Palmer, J., Ghita, O., Savage, L., & Evans, K. E. (2009). Successful closed-loop recycling of thermoset composites. Composites Part A: Applied Science and Manufacturing, 40(4), 490–498. https://doi.org/10.1016/j.compositesa.2009.02.002
[41]Oliveux, G., Dandy, L. O., & Leeke, G. A. (2015). Degradation of a model epoxy resin by solvolysis routes. Polymer Degradation and Stability, 118, 96–103. https://doi.org/10.1016/j.polymdegradstab.2015.04.016
[42]Piñero-Hernanz, R., Dodds, C., Hyde, J., García-Serna, J., Poliakoff, M., Lester, E., Kingman, S., Pickering, S., & Wong, K. H. (2008). Chemical recycling of carbon fibre reinforced composites in nearcritical and supercritical water. Composites Part A: Applied Science and Manufacturing, 39(3), 454–461. https://doi.org/10.1016/j.compositesa.2008.01.001
[43]Liu, Y., Meng, L., Huang, Y., & Du, J. (2004). Recycling of carbon/epoxy composites. Journal of Applied Polymer Science, 94(5), 1912–1916. https://doi.org/10.1002/app.20990
[44]Okajima, I., Hiramatsu, M., Shimamura, Y., Awaya, T., & Sako, T. (2014). Chemical recycling of carbon fiber reinforced plastic using supercritical methanol. The Journal of Supercritical Fluids, 91, 68–76. https://doi.org/10.1016/j.supflu.2014.04.011
[45]Yan, H., Lu, C., Jing, D., Chang, C., Liu, B., & Zhang, X. (2015). Chemical degradation of amine-cured DGEBA epoxy resin in supercritical 1-propanol. Journal of Applied Polymer Science, 132(12), Article 41686.
[46]Das, M., Chacko, R., & Varughese, S. (2018). An efficient method of recycling of CFRP waste using peracetic acid. ACS Sustainable Chemistry & Engineering, 6(2), 1564–1571. https://doi.org/10.1021/acssuschemeng.7b01456
[47]Morin, C., Loppinet-Serani, A., Cansell, F., & Aymonier, C. (2012). Near- and supercritical solvolysis of carbon fibre reinforced polymers (CFRPs) for recycling carbon fibers as a valuable resource: State of the art. The Journal of Supercritical Fluids, 66, 232–240. https://doi.org/10.1016/j.supflu.2012.02.001
[48]Wang, Y., Cui, X., Ge, H., Yang, Y., Wang, Y., Zhang, C., Li, J., Deng, T., Qin, Z., & Hou, X. (2015). Chemical recycling of carbon fiber reinforced epoxy resin composites via selective cleavage of the carbon–nitrogen bond. ACS Sustainable Chemistry & Engineering, 3(12), 3332–3337. https://doi.org/10.1021/acssuschemeng.5b00949
[49]Keith, M. J., Leeke, G. A., & Lester, E. (2010). Supercritical carbon dioxide extraction of hexabromocyclododecane from polymeric materials. Environmental Science & Technology, 44(12), 4570–4575.
[50]Kaufmann, J., Temesgen, A. G., & Cebulla, H. (2025). A comprehensive review on natural fiber reinforced hybrid composites processing techniques, material properties and emerging applications. Discover Materials, 5, Article 227. https://doi.org/10.1007/s43939-025-00419-z
[51]Vo Dong, P. A., Azzaro-Pantel, C., & Cadene, A.-L. (2018). Economic and environmental assessment of recovery and disposal pathways for CFRP waste management. Resources, Conservation and Recycling, 133, 63–75. https://doi.org/10.1016/j.resconrec.2018.01.024
[52]Khalil, Y. F. (2018). Comparative environmental and human health evaluations of thermolysis and solvolysis recycling technologies of carbon fiber reinforced polymer waste. Waste Management, 76, 767–778. https://doi.org/10.1016/j.wasman.2018.03.026
[53]Wong, K. H., Pickering, S. J., & Rudd, C. D. (2010). Recycled carbon fibre reinforced polymer composite for electromagnetic interference shielding. Composites Part A: Applied Science and Manufacturing, 41(6), 693–702. https://doi.org/10.1016/j.compositesa.2010.01.012
[54]Akonda, M. H., Lawrence, C. A., & Weager, B. M. (2012). Recycled carbon fibre-reinforced polypropylene thermoplastic composites. Composites Part A: Applied Science and Manufacturing, 43(1), 79–86. https://doi.org/10.1016/j.compositesa.2011.09.014
[55]Jiang, G., Pickering, S. J., Walker, G. S., Wong, K. H., & Rudd, C. D. (2008). Surface characterisation of carbon fibre recycled using fluidised bed. Applied Surface Science, 254(9), 2588–2593. https://doi.org/10.1016/j.apsusc.2007.09.105
[56]Yuyan, L., Guohua, S., & Linghui, D. (2009). A chemical degradation process for the recycling of epoxy/carbon fiber composites. Composites Science and Technology, 69(2), 264–270.
[57]Turner, T. A., Pickering, S. J., & Warrior, N. A. (2011). Development of recycled carbon fibre moulding compounds—Preparation of waste composites. Composites Part B: Engineering, 42(3), 517–525. https://doi.org/10.1016/j.compositesb.2010.11.010
[58]Yip, H. L. H., Pickering, S. J., & Rudd, C. D. (2002). Characterisation of carbon fibres recycled from scrap composites using fluidised bed process. Plastics, Rubber and Composites, 31(6), 278–282. https://doi.org/10.1179/146580102225003047
[59]Mativenga, P. T., Shuaib, N. A., Howarth, J., Pestalozzi, F., & Woidasky, J. (2016). High voltage fragmentation and mechanical recycling of glass fibre thermoset composite. CIRP Annals, 65(1), 45–48. https://doi.org/10.1016/j.cirp.2016.04.107
[60]Asmatulu, E., Twomey, J., & Overcash, M. (2014). Recycling of fiber-reinforced composites and direct structural composite recycling concept. Journal of Composite Materials, 48(5), 593–608. https://doi.org/10.1177/0021998313476325
[61]Ribeiro, M. C. S., Fiúza, A., Ferreira, A., Dinis, M. D. L., Meira Castro, A. C., Meixedo, J. P., & Alvim, M. R. (2016). Recycling approach towards sustainability advance of composite materials’ industry. Recycling, 1(1), 178–193. https://doi.org/10.3390/recycling1010178
[62]La Rosa, A. D., Recca, G., Summerscales, J., Latteri, A., Cozzo, G., & Cicala, G. (2014). Bio-based versus traditional polymer composites: A life cycle assessment perspective. Journal of Cleaner Production, 74, 135–144. https://doi.org/10.1016/j.jclepro.2014.03.017
[63]Mastali, M., Dalvand, A., & Sattarifard, A. R. (2016). The impact resistance and mechanical properties of reinforced self-compacting concrete with recycled glass fibre reinforced polymers. Journal of Cleaner Production, 124, 312–324. https://doi.org/10.1016/j.jclepro.2016.02.148
[64]Sauer, M. (2019). Composites market report 2019. Carbon Composites, AVK–Industrievereinigung Verstärkte Kunststoffe.
[65]ELG Carbon Fibre Ltd. (2024). Technical documentation. [Unable to independently verify the specific document.].
[66]Ribeiro, I., Kaufmann, J., Schmidt, A., Peças, P., Henriques, E., & Götze, U. (2016). Fostering selection of sustainable manufacturing technologies: A case study involving product design, supply chain and life cycle performance. Journal of Cleaner Production, 112, 3306–3319. https://doi.org/10.1016/j.jclepro.2015.10.043
[67]Meng, F., McKechnie, J., Turner, T. A., & Pickering, S. J. (2017). Energy and environmental assessment and reuse of fluidised bed recycled carbon fibres. Composites Part A: Applied Science and Manufacturing, 100, 206–214. https://doi.org/10.1016/j.compositesa.2017.05.008
[68]Shuaib, N. A., & Mativenga, P. T. (2017). Carbon footprint analysis of fibre reinforced composite recycling processes. Procedia Manufacturing, 7, 183–190. https://doi.org/10.1016/j.promfg.2016.12.046
[69]Metzner, C., Gessler, A., Kaufmann, J., & Kroll, L. (2015). Functionalized braids as potential solution for high performance CFRP structures. In Proceedings of the 2nd International MERGE Technologies Conference (IMTC 2015) (pp. 37–44). Chemnitz University of Technology.
[70]Ribeiro, I., Kaufmann, J., Götze, U., Peças, P., & Henriques, E. (2019). Fibre reinforced polymers in the sports industry: Life Cycle Engineering methodology applied to a snowboard using anisotropic layer design. International Journal of Sustainable Engineering, 12(3), 201–211. https://doi.org/10.1080/19397038.2018.1508318
[71]Carvalho, H., Raposo, A., Ribeiro, I., Kaufmann, J., Götze, U., Peças, P., & Henriques, E. (2016). Application of Life Cycle Engineering approach to assess the pertinence of using natural fibers in composites: The rocker case study. Procedia CIRP, 48, 364–369. https://doi.org/10.1016/j.procir.2016.03.144
[72]Götze, U., Hertel, A., Schmidt, A., Päßler, E., & Kaufmann, J. (2013). Integrated framework for life cycle-oriented evaluation of product and process technologies: Conceptual design and case study. In F. Klocke, B. Döbbeler, M. Binder, R. Schlosser, & D. Lung (Eds.), Technology and manufacturing process selection: The product life cycle perspective (pp. 193–215). Springer. https://doi.org/10.1007/978-1-4471-5544-7_10
[73]Götze, U., Peças, P., Salman, H. M., Kaufmann, J., & Schmidt, A. (2019). Risk-sensitive life cycle assessment of green composites for automotive applications. In G. Koronis & A. Silva (Eds.), Green composites for automotive applications (pp. 219–251). Woodhead Publishing. https://doi.org/10.1016/B978-0-08-102177-4.00010-0
[74]Denissen, W., Winne, J. M., & Du Prez, F. E. (2016). Vitrimers: Permanent organic networks with glass-like fluidity. Chemical Science, 7(1), 30–38. https://doi.org/10.1039/C5SC02223A
[75]Knight, C. (2019). The circular economy and the future of composites. Reinforced Plastics, 63(4), 194–198. [Unable to independently verify the complete bibliographic record.].
[76]Beauson, J., & Brøndsted, P. (2016). Wind turbine blades: An end of life perspective. In W. Ostachowicz, M. McGugan, J.-U. Schröder-Hinrichs, & M. Luczak (Eds.), MARE-WINT: New materials and reliability in offshore wind turbine technology (pp. 421–432). Springer. https://doi.org/10.1007/978-3-319-39095-6_23
[77]Jensen, J. P., & Skelton, K. (2018). Wind turbine blade recycling: Experiences, challenges and possibilities in a circular economy. Renewable and Sustainable Energy Reviews, 97, 165–176. https://doi.org/10.1016/j.rser.2018.08.041
[78]Job, S. (2013). Recycling glass fibre reinforced composites: History and progress. Reinforced Plastics, 57(5), 19–23. https://doi.org/10.1016/S0034-3617(13)70151-6
[79]Liu, P., Meng, F., & Barlow, C. Y. (2019). Wind turbine blade end-of-life options: An eco-audit comparison. Journal of Cleaner Production, 212, 1268–1281. https://doi.org/10.1016/j.jclepro.2018.12.043
[80]Rani, M., Choudhary, P., Krishnan, V., & Zafar, S. (2021). A review on recycling and reuse methods for carbon fiber/glass fiber composites waste from wind turbine blades. Composites Part B: Engineering, 215, Article 108768. https://doi.org/10.1016/j.compositesb.2021.108768

This work is licensed under a Creative Commons Attribution 4.0 International License.
View
PDF
How to Cite